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NAND flash memory-based SSDs have been widely adopted. The scaling of SSD has evolved from plannar (2D) to 3D stacking. For reliability and other reasons, the technology node in 3D NAND SSD is larger than in 2D, but data density can be increased via increasing bit-per-cell. In this work, we develop a novel reprogramming scheme for TLCs in 3D NAND SSD, such that a cell can be programmed and reprogrammed several times before it is erased. Such reprogramming can improve the endurance of a cell and the speed of programming, and increase the amount of bits written in a cell per program/erase cycle, i.e., effective capacity. Our work is the first to perform a real 3D NAND SSD test to validate the feasibility of the reprogram operation. From the collected data, we derive the restrictions of performing reprogramming due to reliability challenges. Furthermore, a reprogrammable SSD (ReSSD) is designed to structure reprogram operations. ReSSD is evaluated in a case study in RAID 5 system (RSS-RAID). Experimental results show that RSS-RAID can improve the endurance by 35.7%, boost write performance by 15.9%, and increase effective capacity by 7.71%, with negligible overhead compared with conventional 3D SSD-based RAID 5 system. 

Including both environmental and vibronic effects is important for accurate simulation of optical spectra, but combining these effects remains computationally challenging. We outline two approaches that consider both the explicit atomistic environment and the vibronic transitions. Both phenomena are responsible for spectral shapes in linear spectroscopy and the electronic evolution measured in nonlinear spectroscopy. The first approach utilizes snapshots of chromophore-environment configurations for which chromophore normal modes are determined. We outline various approximations for this static approach that assumes harmonic potentials and ignores dynamic system-environment coupling. The second approach obtains excitation energies for a series of time-correlated snapshots. This dynamic approach relies on the accurate truncation of the cumulant expansion but treats the dynamics of the chromophore and the environment on equal footing. Both approaches show significant potential for making strides toward more accurate optical spectroscopy simulations of complex condensed phase systems.